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Parameters optimization for eutrophic lake water treatment by a novel process of iron-carbon micro-electrolysis coupled with catalytic ozonation using response surface methodology
A novel process of iron-carbon micro-electrolysis (ICME) coupled with catalytic ozonation (CO) for treatment of eutrophic lake water was developed. A series of batch experiments with ICME alone and CO alone was designed to investigate the effects of process parameters, such as initial pH, dose of Fe-C, time of micro-electrolysis, ozone flux, dose of TiO2/activated carbon (TiO2/AC), and time of ozonation, on the removal rates of total nitrogen (TN), total phosphorus (TP), CODMn and Chl-a. The process parameters were optimized using response surface methodology. The results showed that initial pH, dose of Fe-C and ozone flux had significant effects on removal of TN, TP, CODMn and Chl-a. Within the range of selected operating conditions, the optimized values of initial pH, dose of Fe-C, time of micro-electrolysis, ozone flux, dose of TiO2/AC, and time of ozonation were 3.8, 13.7 g/L, 29.6 min, 3.19 L/min, 294.74 mg/L and 106.73 min, respectively. Furthermore, ICME alone had significant advantages in TP and CODMn removal and CO alone favored TN and Chl-a. Under the optimal process conditions, the final removal rates of TN, TP, CODMn, and Chl-a by the hybrid ICME-CO process reached 75.33%, 86.29%, 94.42% and 97.57%, respectively. The present research provides a new alternative technology with promise for treatment of eutrophic lake water. HIGHLIGHTS A novel coupling ICME-CO process was developed for treatment of eutrophic water.; Six process parameters were optimized using RSM.; Initial pH, dose of Fe-C and ozone flux had significant effects on removal of various pollutants.; The final removal rates for TN, TP, CODMn, and Chl-a by the ICME-CO process reached 75.33%, 86.29%, 94.42% and 97.57%.;
Parameters optimization for eutrophic lake water treatment by a novel process of iron-carbon micro-electrolysis coupled with catalytic ozonation using response surface methodology
A novel process of iron-carbon micro-electrolysis (ICME) coupled with catalytic ozonation (CO) for treatment of eutrophic lake water was developed. A series of batch experiments with ICME alone and CO alone was designed to investigate the effects of process parameters, such as initial pH, dose of Fe-C, time of micro-electrolysis, ozone flux, dose of TiO2/activated carbon (TiO2/AC), and time of ozonation, on the removal rates of total nitrogen (TN), total phosphorus (TP), CODMn and Chl-a. The process parameters were optimized using response surface methodology. The results showed that initial pH, dose of Fe-C and ozone flux had significant effects on removal of TN, TP, CODMn and Chl-a. Within the range of selected operating conditions, the optimized values of initial pH, dose of Fe-C, time of micro-electrolysis, ozone flux, dose of TiO2/AC, and time of ozonation were 3.8, 13.7 g/L, 29.6 min, 3.19 L/min, 294.74 mg/L and 106.73 min, respectively. Furthermore, ICME alone had significant advantages in TP and CODMn removal and CO alone favored TN and Chl-a. Under the optimal process conditions, the final removal rates of TN, TP, CODMn, and Chl-a by the hybrid ICME-CO process reached 75.33%, 86.29%, 94.42% and 97.57%, respectively. The present research provides a new alternative technology with promise for treatment of eutrophic lake water. HIGHLIGHTS A novel coupling ICME-CO process was developed for treatment of eutrophic water.; Six process parameters were optimized using RSM.; Initial pH, dose of Fe-C and ozone flux had significant effects on removal of various pollutants.; The final removal rates for TN, TP, CODMn, and Chl-a by the ICME-CO process reached 75.33%, 86.29%, 94.42% and 97.57%.;
Parameters optimization for eutrophic lake water treatment by a novel process of iron-carbon micro-electrolysis coupled with catalytic ozonation using response surface methodology
Shanqing Jiang (Autor:in) / Yu Cao (Autor:in) / Pei Han (Autor:in) / Yanan Zhang (Autor:in) / Hankun Zhang (Autor:in) / Qiuya Zhang (Autor:in) / Xia Xu (Autor:in) / Yuanyuan Zhou (Autor:in) / Liping Wang (Autor:in)
2021
Aufsatz (Zeitschrift)
Elektronische Ressource
Unbekannt
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