Below-cloud scavenging of aerosol particles by precipitation in a typical valley city, northwestern China: Fid-Bau Portal

Below-cloud scavenging of aerosol particles by precipitation in a typical valley city, northwestern China

Zhao, Suping / Yu, Ye / He, Jianjun / Yin, Daiying / Wang, Bo

Abstract To fill the blank information for aerosol precipitation-scavenging research in north-west of China, the aerosol particle and raindrop size distributions were measured simultaneously during 1 September 2012 to 31 August 2013 in urban Lanzhou. The scavenging coefficients of thunderstorm and non-thunderstorm rain and snow events were studied and presented on the basis of nine selected precipitation cases including 3 snow and 6 rain events. The variation of scavenging coefficients of snowfall across the size distribution clearly exhibited a trough of lower values for particles of 1000 nm–2000 nm in diameter, while the particles smaller than 500 nm were scavenged efficiently by non-thunderstorm rain, and thunderstorm rain more effectively scavenged the particles in 500–1000 nm. The snow scavenging coefficients varied between 3.11 × 10⁻⁷ s⁻¹ and 1.18 × 10⁻³ s⁻¹ in the 10–10,000 nm size range. The scavenging coefficients of thunderstorm (non-thunderstorm) rain were between 8.25 × 10⁻⁷ s⁻¹ (7.48 × 10⁻⁶ s⁻¹) and 1.23 × 10⁻³ s⁻¹ (7.46 × 10⁻⁴ s⁻¹). Additionally, the number of particles in 10–50 nm was more sensitive to duration of snow, while snowfall intensity was more responsible for particle number concentrations in 50–100 nm and 100–1000 nm. The longer period of precipitation with lower raindrop velocity can more effectively scavenge the particles in the size range of 10–50 nm.

Highlights • Scavenging effects of rain and snow on aerosol particles were evaluated. • Snow scavenged particles in 20–1000 nm and 2000–10,000 nm more efficiently than rain. • The thunderstorm rain more efficiently scavenged the particles in 500–1000 nm. • Duration and raindrop velocity were main factors affecting aerosol particles.