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Impacts of variations in aerosol refractive index on the retrieving of the light-absorption and hygroscopicity of ambient black carbon-containing aerosols using SP2
https://orcid.org/0000-0001-7160-4600
https://orcid.org/0000-0003-1951-379X
Abstract Black carbon (BC) aerosols directly influence the earth's climate system by absorbing the light intensity and indirectly by interacting with clouds. The microphysical properties of BC-containing aerosols were determined by their core diameter and shell thickness, which can be derived from the measurement of a single-particle soot photometer (SP2). Traditionally, a constant real part of the shell's refractive index (RRI) was employed to retrieve the shell thickness of BC-containing aerosols using the measured scattering signals from SP2. Recent field measurements in East China show that ambient aerosol RRI varies over a wide range between 1.36 and 1.56. The influences of aerosol RRI variation on the retrieving of BC-containing aerosol shell thickness from the measurements of SP2 are investigated with simulation studies. Results show that the variation in ambient aerosol RRI can lead to a variation in the coating thickness of BC-containing aerosols by 9.4%. The corresponding uncertainties in the light absorption enhancement reach up to 29% due to the influence of aerosol RRI. The critical mean supersaturation (SS) of the BC-containing aerosol varies significantly between 0.044% and 0.055% due to the uncertainties in the derived shell thickness using a constant RRI. This study highlights the demand for the real-time measurement of ambient aerosol RRI when deriving the microphysical properties of ambient BC-containing aerosols from the SP2 measurement.
Highlights Influence of the variation in aerosol refractive index on the microphysical properties of SP2-measured BC was estimated. Coating thickness of BC would vary by 9.4% due to the variation in the black carbon coating’s refractive index. The light absorption ability would vary by 29% due to the influence of the aerosol coating's refractive index.
Impacts of variations in aerosol refractive index on the retrieving of the light-absorption and hygroscopicity of ambient black carbon-containing aerosols using SP2
https://orcid.org/0000-0001-7160-4600
https://orcid.org/0000-0003-1951-379X
Abstract Black carbon (BC) aerosols directly influence the earth's climate system by absorbing the light intensity and indirectly by interacting with clouds. The microphysical properties of BC-containing aerosols were determined by their core diameter and shell thickness, which can be derived from the measurement of a single-particle soot photometer (SP2). Traditionally, a constant real part of the shell's refractive index (RRI) was employed to retrieve the shell thickness of BC-containing aerosols using the measured scattering signals from SP2. Recent field measurements in East China show that ambient aerosol RRI varies over a wide range between 1.36 and 1.56. The influences of aerosol RRI variation on the retrieving of BC-containing aerosol shell thickness from the measurements of SP2 are investigated with simulation studies. Results show that the variation in ambient aerosol RRI can lead to a variation in the coating thickness of BC-containing aerosols by 9.4%. The corresponding uncertainties in the light absorption enhancement reach up to 29% due to the influence of aerosol RRI. The critical mean supersaturation (SS) of the BC-containing aerosol varies significantly between 0.044% and 0.055% due to the uncertainties in the derived shell thickness using a constant RRI. This study highlights the demand for the real-time measurement of ambient aerosol RRI when deriving the microphysical properties of ambient BC-containing aerosols from the SP2 measurement.
Highlights Influence of the variation in aerosol refractive index on the microphysical properties of SP2-measured BC was estimated. Coating thickness of BC would vary by 9.4% due to the variation in the black carbon coating’s refractive index. The light absorption ability would vary by 29% due to the influence of the aerosol coating's refractive index.
Impacts of variations in aerosol refractive index on the retrieving of the light-absorption and hygroscopicity of ambient black carbon-containing aerosols using SP2
https://orcid.org/0000-0001-7160-4600
https://orcid.org/0000-0003-1951-379X
Abstract Black carbon (BC) aerosols directly influence the earth's climate system by absorbing the light intensity and indirectly by interacting with clouds. The microphysical properties of BC-containing aerosols were determined by their core diameter and shell thickness, which can be derived from the measurement of a single-particle soot photometer (SP2). Traditionally, a constant real part of the shell's refractive index (RRI) was employed to retrieve the shell thickness of BC-containing aerosols using the measured scattering signals from SP2. Recent field measurements in East China show that ambient aerosol RRI varies over a wide range between 1.36 and 1.56. The influences of aerosol RRI variation on the retrieving of BC-containing aerosol shell thickness from the measurements of SP2 are investigated with simulation studies. Results show that the variation in ambient aerosol RRI can lead to a variation in the coating thickness of BC-containing aerosols by 9.4%. The corresponding uncertainties in the light absorption enhancement reach up to 29% due to the influence of aerosol RRI. The critical mean supersaturation (SS) of the BC-containing aerosol varies significantly between 0.044% and 0.055% due to the uncertainties in the derived shell thickness using a constant RRI. This study highlights the demand for the real-time measurement of ambient aerosol RRI when deriving the microphysical properties of ambient BC-containing aerosols from the SP2 measurement.
Highlights Influence of the variation in aerosol refractive index on the microphysical properties of SP2-measured BC was estimated. Coating thickness of BC would vary by 9.4% due to the variation in the black carbon coating’s refractive index. The light absorption ability would vary by 29% due to the influence of the aerosol coating's refractive index.
Impacts of variations in aerosol refractive index on the retrieving of the light-absorption and hygroscopicity of ambient black carbon-containing aerosols using SP2
Zhao, Gang (Autor:in) / Hu, Min (Autor:in) / Zhao, Chunsheng (Autor:in)
Atmospheric Environment ; 321
17.01.2024
Aufsatz (Zeitschrift)
Elektronische Ressource
Englisch
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