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Polycyclic aromatic hydrocarbons and polybrominated diphenyl ethers inside university campus: Indoor dust-bound pollution characteristics and health risks to university student
Abstract This study examined indoor dust-bound pollution characteristics of polycyclic aromatic hydrocarbons (PAHs) and polybrominated diphenyl ethers (PBDEs), and the health risk to these pollutants of university students inside a university campus in Xinxiang, central China. Indoor dust samples (n = 52) were obtained from the student dormitories, classrooms, laboratories, and offices. The average concentration of ∑16PAHs was 2060 ± 1290 ng/g dry weight (dw). Phe and 4-ring PAHs showed the highest concentration and contribution. The PAH concentrations in indoor dust from various types of room showed significant difference (p ˂ 0.05), and the highest concentration was found in laboratory. The ∑16PBDEs concentration was 364 ± 379 ng/g, and BDE209 was the prime PBDE congener and showed the highest contribution. PBDE concentrations also showed significant difference (p ˂ 0.05) among different types of indoor dust, and the girls’ dormitory showed the highest PBDEs concentration. Petroleum, petroleum combustion, and biomass/coal combustion were the main sources of PAHs. Deca-BDE (BDE209) was the main source of PBDEs, and low-brominated PBDEs were mainly derived from the degradation of high-brominated PBDEs. Correlation analysis showed that PAH and PBDE had similar pollution sources. The estimated daily intake (EDIs, mg/(kg·day)) of the ∑16PAHs was 694 ± 434. The BaP equivalent (BaPE) value for PAHs in indoor dust was 113 ng/g, and laboratory showed the highest BaPE values. The EDIs of the ∑16PBDEs were 123 ± 128 mg/(kg·day), and the non-cancer hazard index (HI) indicated PBDEs may pose adverse health effects to university students.
Graphical abstract Display Omitted
Highlights PAHs and PBDEs in different types of indoor dust showed significant difference. 4-ring PAHs and BDE 209 showed the highest value and contribution. PAHs and PBDEs were significantly correlated, and may have similar origins. Indoor dust-bound PBDEs posed high potential health risks to university students.
Polycyclic aromatic hydrocarbons and polybrominated diphenyl ethers inside university campus: Indoor dust-bound pollution characteristics and health risks to university student
Abstract This study examined indoor dust-bound pollution characteristics of polycyclic aromatic hydrocarbons (PAHs) and polybrominated diphenyl ethers (PBDEs), and the health risk to these pollutants of university students inside a university campus in Xinxiang, central China. Indoor dust samples (n = 52) were obtained from the student dormitories, classrooms, laboratories, and offices. The average concentration of ∑16PAHs was 2060 ± 1290 ng/g dry weight (dw). Phe and 4-ring PAHs showed the highest concentration and contribution. The PAH concentrations in indoor dust from various types of room showed significant difference (p ˂ 0.05), and the highest concentration was found in laboratory. The ∑16PBDEs concentration was 364 ± 379 ng/g, and BDE209 was the prime PBDE congener and showed the highest contribution. PBDE concentrations also showed significant difference (p ˂ 0.05) among different types of indoor dust, and the girls’ dormitory showed the highest PBDEs concentration. Petroleum, petroleum combustion, and biomass/coal combustion were the main sources of PAHs. Deca-BDE (BDE209) was the main source of PBDEs, and low-brominated PBDEs were mainly derived from the degradation of high-brominated PBDEs. Correlation analysis showed that PAH and PBDE had similar pollution sources. The estimated daily intake (EDIs, mg/(kg·day)) of the ∑16PAHs was 694 ± 434. The BaP equivalent (BaPE) value for PAHs in indoor dust was 113 ng/g, and laboratory showed the highest BaPE values. The EDIs of the ∑16PBDEs were 123 ± 128 mg/(kg·day), and the non-cancer hazard index (HI) indicated PBDEs may pose adverse health effects to university students.
Graphical abstract Display Omitted
Highlights PAHs and PBDEs in different types of indoor dust showed significant difference. 4-ring PAHs and BDE 209 showed the highest value and contribution. PAHs and PBDEs were significantly correlated, and may have similar origins. Indoor dust-bound PBDEs posed high potential health risks to university students.
Polycyclic aromatic hydrocarbons and polybrominated diphenyl ethers inside university campus: Indoor dust-bound pollution characteristics and health risks to university student
Wu, Zhineng (Autor:in) / Lyu, Honghong (Autor:in) / Guo, Ying (Autor:in) / Man, Quanli (Autor:in) / Niu, Hanyu (Autor:in) / Li, Junyi (Autor:in) / Jing, Xiaohua (Autor:in) / Ren, Gengbo (Autor:in) / Ma, Xiaodong (Autor:in)
Building and Environment ; 221
14.06.2022
Aufsatz (Zeitschrift)
Elektronische Ressource
Englisch
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