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Colloidal Quantum Dot Light-Emitting Diodes Employing Phosphorescent Small Organic Molecules as Efficient Exciton Harvesters
The authors would like to acknowledge the financial support from the Singapore National Research Foundation under the programs of NRF-RF-2009-09 and NRF-CRP-6-2010-02, the Science and Engineering Research Council, Agency for Science, Technology and Research (A*STAR) of Singapore (Project Nos. 61006037 and 61076015), EU-FP7 Nanophotonics4-Energy NoE, TUBITAK EEEAG 109E002, 109E004, 110E010, 110E217, ESF-EURYI, and TUBA-GEBIP. E.M. acknowledges BAGEP award ; Nonradiative energy transfer (NRET) is an alternative excitation mechanism in colloidal quantum dot (QD) based electroluminescent devices (QLEDs). Here, we develop hybrid highly spectrally pure QLEDs that facilitate energy transfer pumping via NRET from a phosphorescent small organic molecule-codoped charge transport layer to the adjacent QDs. A partially codoped exciton funnelling electron transport layer is proposed and optimized for enhanced QLED performance while exhibiting very high color purity of 99%. These energy transfer pumped hybrid QLEDs demonstrate a 6-fold enhancement factor in the external quantum efficiency over the conventional QLED structure, in which energy transfer pumping is intrinsically weak. ; Singapore National Research Foundation NRF-RF-2009-09 NRF-CRP-6-2010-02 Agency for Science Technology & Research (ASTAR) 61006037 61076015 Turkiye Bilimsel ve Teknolojik Arastirma Kurumu (TUBITAK) 109E002 109E004 110E010 110E217 European Science Foundation (ESF) Turkish Academy of Sciences BAGEP award Science and Engineering Research Council EU-FP7 Nanophotonics4-Energy NoE
Colloidal Quantum Dot Light-Emitting Diodes Employing Phosphorescent Small Organic Molecules as Efficient Exciton Harvesters
The authors would like to acknowledge the financial support from the Singapore National Research Foundation under the programs of NRF-RF-2009-09 and NRF-CRP-6-2010-02, the Science and Engineering Research Council, Agency for Science, Technology and Research (A*STAR) of Singapore (Project Nos. 61006037 and 61076015), EU-FP7 Nanophotonics4-Energy NoE, TUBITAK EEEAG 109E002, 109E004, 110E010, 110E217, ESF-EURYI, and TUBA-GEBIP. E.M. acknowledges BAGEP award ; Nonradiative energy transfer (NRET) is an alternative excitation mechanism in colloidal quantum dot (QD) based electroluminescent devices (QLEDs). Here, we develop hybrid highly spectrally pure QLEDs that facilitate energy transfer pumping via NRET from a phosphorescent small organic molecule-codoped charge transport layer to the adjacent QDs. A partially codoped exciton funnelling electron transport layer is proposed and optimized for enhanced QLED performance while exhibiting very high color purity of 99%. These energy transfer pumped hybrid QLEDs demonstrate a 6-fold enhancement factor in the external quantum efficiency over the conventional QLED structure, in which energy transfer pumping is intrinsically weak. ; Singapore National Research Foundation NRF-RF-2009-09 NRF-CRP-6-2010-02 Agency for Science Technology & Research (ASTAR) 61006037 61076015 Turkiye Bilimsel ve Teknolojik Arastirma Kurumu (TUBITAK) 109E002 109E004 110E010 110E217 European Science Foundation (ESF) Turkish Academy of Sciences BAGEP award Science and Engineering Research Council EU-FP7 Nanophotonics4-Energy NoE
Colloidal Quantum Dot Light-Emitting Diodes Employing Phosphorescent Small Organic Molecules as Efficient Exciton Harvesters
Mutlugun, Evren (author) / Guzelturk, Burak (author) / Abiyasa, Agus Putu (author) / Gao, Yuan (author) / Sun, Xiao Wei (author) / Demir, Hilmi Volkan (author) / AGÜ, Mühendislik Fakültesi, Elektrik & Elektronik Mühendisliği Bölümü
2014-01-01
Article (Journal)
Electronic Resource
English
DDC:
690
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