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Role of traffic in atmospheric accumulation of heavy metals and polycyclic aromatic hydrocarbons
Abstract Traffic related emissions have been recognised as one of the main sources of air pollutants. In the research study discussed in this paper, variability of atmospheric total suspended particulate matter (TSP), polycyclic aromatic hydrocarbons (PAH) and heavy metal (HM) concentrations with traffic and land use characteristics during weekdays and weekends were investigated. Data required for the study were collected from a range of sampling sites to ensure a wide mix of traffic and land use characteristics. The analysis undertaken confirmed that zinc has the highest concentration in the atmospheric phase during weekends as well as weekdays. Although the use of leaded gasoline was discontinued a decade ago, lead was the second most commonly detected heavy metal. This is attributed to the association of previously generated lead with roadside soil and re-suspension to the atmosphere. Soil related particles are the primary source of TSP and manganese to the atmosphere. The analysis further revealed that traffic sources are dominant in gas phase PAHs compared to the other sources during weekdays. Land use related sources become important contributors to atmospheric PAHs during weekends when traffic sources are at their minimal levels.
Highlights ► Role of traffic in atmospheric accumulation of heavy metals and PAHs investigated. ► Zinc has the highest concentration during weekends as well as weekdays. ► Re-suspension of roadside soil result in lead being second commonly detected metal. ► Soil particles are the primary source of TSP and manganese to the atmosphere. ► Traffic sources are dominant in gas phase PAHs during weekdays.
Role of traffic in atmospheric accumulation of heavy metals and polycyclic aromatic hydrocarbons
Abstract Traffic related emissions have been recognised as one of the main sources of air pollutants. In the research study discussed in this paper, variability of atmospheric total suspended particulate matter (TSP), polycyclic aromatic hydrocarbons (PAH) and heavy metal (HM) concentrations with traffic and land use characteristics during weekdays and weekends were investigated. Data required for the study were collected from a range of sampling sites to ensure a wide mix of traffic and land use characteristics. The analysis undertaken confirmed that zinc has the highest concentration in the atmospheric phase during weekends as well as weekdays. Although the use of leaded gasoline was discontinued a decade ago, lead was the second most commonly detected heavy metal. This is attributed to the association of previously generated lead with roadside soil and re-suspension to the atmosphere. Soil related particles are the primary source of TSP and manganese to the atmosphere. The analysis further revealed that traffic sources are dominant in gas phase PAHs compared to the other sources during weekdays. Land use related sources become important contributors to atmospheric PAHs during weekends when traffic sources are at their minimal levels.
Highlights ► Role of traffic in atmospheric accumulation of heavy metals and PAHs investigated. ► Zinc has the highest concentration during weekends as well as weekdays. ► Re-suspension of roadside soil result in lead being second commonly detected metal. ► Soil particles are the primary source of TSP and manganese to the atmosphere. ► Traffic sources are dominant in gas phase PAHs during weekdays.
Role of traffic in atmospheric accumulation of heavy metals and polycyclic aromatic hydrocarbons
Gunawardena, Janaka (author) / Egodawatta, Prasanna (author) / Ayoko, Godwin A. (author) / Goonetilleke, Ashantha (author)
Atmospheric Environment ; 54 ; 502-510
2012-02-15
9 pages
Article (Journal)
Electronic Resource
English
Leaching of polycyclic aromatic hydrocarbons and heavy metals from stored reclaimed asphalt pavement
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