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Generation and growth of aerosols over Pune, India
AbstractThe measured physical size distributions of sub-micron particles during cold season at Pune, India are analyzed to explore the characteristics of nucleation and growth properties. Preliminary analysis of aerosol size distribution in time-series shows large increase in number concentration due to nucleation events between 0800h and 1030h at this location. The observable quantities such as condensable vapor concentration (C), its source rate (Q), growth rate (GR) and condensable sink (CS) are estimated from the time-series evolutions of aerosol size distributions. The concentration of vapor and its source rate were about 19.8±2.15×107 moleculescm−3 and 1.28±0.084×107cm−3s−1 respectively. The average condensation sink and growth rate were 7.1±0.4×10−2s−1 and 16.95±1.86nmh−1 respectively during the growth period. The values are high enough to trigger the nucleation bursts and enhance subsequent growth rates of nucleation mode particles at this location. The magnitudes are in the range of those observed at New Delhi, India and much higher than those of European cities. The ratio of apparent to real nucleation rate is found to be a measure of number concentration of freshly produced particles by photo-chemical nucleation. The predicted number concentrations corresponding to measured distributions of mid-point diameter increases with the size for both 1nm nucleated clusters and 3nm particles. The database of all the possible event days and the event characteristics forms the basis for future works into the causes and implications of atmospheric particle formation at this location.
Generation and growth of aerosols over Pune, India
AbstractThe measured physical size distributions of sub-micron particles during cold season at Pune, India are analyzed to explore the characteristics of nucleation and growth properties. Preliminary analysis of aerosol size distribution in time-series shows large increase in number concentration due to nucleation events between 0800h and 1030h at this location. The observable quantities such as condensable vapor concentration (C), its source rate (Q), growth rate (GR) and condensable sink (CS) are estimated from the time-series evolutions of aerosol size distributions. The concentration of vapor and its source rate were about 19.8±2.15×107 moleculescm−3 and 1.28±0.084×107cm−3s−1 respectively. The average condensation sink and growth rate were 7.1±0.4×10−2s−1 and 16.95±1.86nmh−1 respectively during the growth period. The values are high enough to trigger the nucleation bursts and enhance subsequent growth rates of nucleation mode particles at this location. The magnitudes are in the range of those observed at New Delhi, India and much higher than those of European cities. The ratio of apparent to real nucleation rate is found to be a measure of number concentration of freshly produced particles by photo-chemical nucleation. The predicted number concentrations corresponding to measured distributions of mid-point diameter increases with the size for both 1nm nucleated clusters and 3nm particles. The database of all the possible event days and the event characteristics forms the basis for future works into the causes and implications of atmospheric particle formation at this location.
Generation and growth of aerosols over Pune, India
Murugavel, P. (author) / Chate, D.M. (author)
Atmospheric Environment ; 43 ; 820-828
2008-10-25
9 pages
Article (Journal)
Electronic Resource
English
Online Contents | 2016
|Elsevier | 2016
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