Catalytic Materials Based on Hydrotalcite-Like Aluminum, Magnesium, Nickel, and Cobalt Hydroxides: Effect of the Nickel/Cobalt Ratio on the Results of Partial Oxidation and Dry Reforming of Methane to Synthesis Gas: Fid-Bau Portal

Catalytic Materials Based on Hydrotalcite-Like Aluminum, Magnesium, Nickel, and Cobalt Hydroxides: Effect of the Nickel/Cobalt Ratio on the Results of Partial Oxidation and Dry Reforming of Methane to Synthesis Gas

Dedov, A. G. / Loktev, A. S. / Danilov, V. P. / Krasnobaeva, O. N. / Nosova, T. A. / Mukhin, I. E. / Baranchikov, A. E. / Yorov, Kh. E. / Bykov, M. A. / Moiseev, I. I.

Abstract

Catalysts for the partial oxidation and dry reforming of methane based on hydroxo salts [AlMg₂Ni_xCo_y(OH)_6.08][(NO₃) ⋅ nH₂O], where x, y = 0, 0.005, 0.01, 0.02, 0.03, 0.035, and 0.04, with a hydrotalcite-like structure and a total Ni and/or Co content of no more than 2 wt % have been synthesized. It has been shown that Ni–Co catalysts with x = 0.03–0.035 and y = 0.005–0.01 provide a synthesis gas yield of 97–99% in both processes. At a low cobalt loading, the catalysts hardly form carbon nanotubes or other carbon depos-its.

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Dedov, A. G. / Loktev, A. S. / Danilov, V. P. / Krasnobaeva, O. N. / Nosova, T. A. / Mukhin, I. E. / Baranchikov, A. E. / Yorov, Kh. E. / Bykov, M. A. / Moiseev, I. I.

Abstract

Dedov, A. G. / Loktev, A. S. / Danilov, V. P. / Krasnobaeva, O. N. / Nosova, T. A. / Mukhin, I. E. / Baranchikov, A. E. / Yorov, Kh. E. / Bykov, M. A. / Moiseev, I. I.