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Methane conversion to valuable chemicals over nanostructured Mo/ZSM-5 catalysts

Ismagilov, Z. R. / Matus, E. V. / Kerzhentsev, M. A. / Tsikoza, L. T. / Ismagilov, I. Z. / Dosumov, K. D. / Mustafin, A. G.

Abstract Results of the ongoing study of nonoxidative methane dehydroaromatization (DHA) over Mo/ZSM-5 catalysts have been analyzed. The effects of the composition, preparation procedure, pretreatment, and the CH4 DHA reaction conditions on the physicochemical and catalytic properties of Mo/ZSM-5 catalysts have been discussed. The data on Mo-containing active sites, the methane DHA reaction mechanism, and the nature of carbonaceous deposits have been considered. The principal causes of the deactivation of Mo/ZSM-5 catalysts and means of their regeneration have been revealed. Approaches to the improvement of the methane DHA process and trends of its further development have been detailed.

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Methane conversion to valuable chemicals over nanostructured Mo/ZSM-5 catalysts

Ismagilov, Z. R. / Matus, E. V. / Kerzhentsev, M. A. / Tsikoza, L. T. / Ismagilov, I. Z. / Dosumov, K. D. / Mustafin, A. G.

Abstract Results of the ongoing study of nonoxidative methane dehydroaromatization (DHA) over Mo/ZSM-5 catalysts have been analyzed. The effects of the composition, preparation procedure, pretreatment, and the CH4 DHA reaction conditions on the physicochemical and catalytic properties of Mo/ZSM-5 catalysts have been discussed. The data on Mo-containing active sites, the methane DHA reaction mechanism, and the nature of carbonaceous deposits have been considered. The principal causes of the deactivation of Mo/ZSM-5 catalysts and means of their regeneration have been revealed. Approaches to the improvement of the methane DHA process and trends of its further development have been detailed.

Methane conversion to valuable chemicals over nanostructured Mo/ZSM-5 catalysts

Ismagilov, Z. R. / Matus, E. V. / Kerzhentsev, M. A. / Tsikoza, L. T. / Ismagilov, I. Z. / Dosumov, K. D. / Mustafin, A. G.

Abstract Results of the ongoing study of nonoxidative methane dehydroaromatization (DHA) over Mo/ZSM-5 catalysts have been analyzed. The effects of the composition, preparation procedure, pretreatment, and the CH4 DHA reaction conditions on the physicochemical and catalytic properties of Mo/ZSM-5 catalysts have been discussed. The data on Mo-containing active sites, the methane DHA reaction mechanism, and the nature of carbonaceous deposits have been considered. The principal causes of the deactivation of Mo/ZSM-5 catalysts and means of their regeneration have been revealed. Approaches to the improvement of the methane DHA process and trends of its further development have been detailed.

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Title:

Methane conversion to valuable chemicals over nanostructured Mo/ZSM-5 catalysts

Contributors:

Ismagilov, Z. R. (author) / Matus, E. V. (author) / Kerzhentsev, M. A. (author) / Tsikoza, L. T. (author) / Ismagilov, I. Z. (author) / Dosumov, K. D. (author) / Mustafin, A. G. (author)

Published in:

Petroleum Chemistry ; 51 ; 174-186

Publication date:

2011-05-01

Size:

13 pages

ISSN:

1555-6239 , 0965-5441

DOI:

https://doi.org/10.1134/S0965544111020058

Type of media:

Article (Journal)

Type of material:

Electronic Resource

Language:

English

Keywords:

Zeolite , High Resolution Transmission Elec Tron Microscopy , Petroleum Chemistry , Methane Conversion , Molybdenum Oxide Chemistry , Industrial Chemistry/Chemical Engineering

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