Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO<sub>2</sub>/CO/H<sub>2</sub>: Fid-Bau Portal

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Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Schmitz, M. / Erken, C. / Ohligschläger, A. / Schnoor, J.‐K. / Westhues, N. F. / Klankermayer, J. / Leitner, W. / Liauw, M. A.

A detailed overview for homogeneously catalyzed strategies and synthesis pathways using a combination of CO₂, CO, and H₂ as active building blocks to selectively obtain C1–C4 alcohols is presented. Conceptual strategies applying homologation, carbonylation, hydrocarboxylation, and hydrogenation reactions will be discussed, finally combining the individual reaction approaches towards potential new pathways to the envisaged alcohol products. Also, tailored reactor concepts with adapted recycling/separation methods for the molecular catalyst systems will be shown and discussed.

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Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Schmitz, M. / Erken, C. / Ohligschläger, A. / Schnoor, J.‐K. / Westhues, N. F. / Klankermayer, J. / Leitner, W. / Liauw, M. A.

A detailed overview for homogeneously catalyzed strategies and synthesis pathways using a combination of CO₂, CO, and H₂ as active building blocks to selectively obtain C1–C4 alcohols is presented. Conceptual strategies applying homologation, carbonylation, hydrocarboxylation, and hydrogenation reactions will be discussed, finally combining the individual reaction approaches towards potential new pathways to the envisaged alcohol products. Also, tailored reactor concepts with adapted recycling/separation methods for the molecular catalyst systems will be shown and discussed.

Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Schmitz, M. / Erken, C. / Ohligschläger, A. / Schnoor, J.‐K. / Westhues, N. F. / Klankermayer, J. / Leitner, W. / Liauw, M. A.

A detailed overview for homogeneously catalyzed strategies and synthesis pathways using a combination of CO₂, CO, and H₂ as active building blocks to selectively obtain C1–C4 alcohols is presented. Conceptual strategies applying homologation, carbonylation, hydrocarboxylation, and hydrogenation reactions will be discussed, finally combining the individual reaction approaches towards potential new pathways to the envisaged alcohol products. Also, tailored reactor concepts with adapted recycling/separation methods for the molecular catalyst systems will be shown and discussed.

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Titel:

Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Beteiligte:

Schmitz, M. (Autor:in) / Erken, C. (Autor:in) / Ohligschläger, A. (Autor:in) / Schnoor, J.‐K. (Autor:in) / Westhues, N. F. (Autor:in) / Klankermayer, J. (Autor:in) / Leitner, W. (Autor:in) / Liauw, M. A. (Autor:in)

Erschienen in:

Chemie Ingenieur Technik ; 90 ; 1476-1488

Erscheinungsdatum:

01.10.2018

Format / Umfang:

13 pages

ISSN:

0009-286X , 1522-2640

DOI:

https://doi.org/10.1002/cite.201800053

Medientyp:

Aufsatz (Zeitschrift)

Format:

Elektronische Ressource

Sprache:

Englisch

Schlagwörter:

Carbon2Chem® , Homogeneous catalysis , (Reverse) Water‐gas shift reaction , Alcohols , Carbon dioxide

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