Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO<sub>2</sub>/CO/H<sub>2</sub>: Fid-Bau Portal

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Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Schmitz, M. / Erken, C. / Ohligschläger, A. / Schnoor, J.‐K. / Westhues, N. F. / Klankermayer, J. / Leitner, W. / Liauw, M. A.

A detailed overview for homogeneously catalyzed strategies and synthesis pathways using a combination of CO₂, CO, and H₂ as active building blocks to selectively obtain C1–C4 alcohols is presented. Conceptual strategies applying homologation, carbonylation, hydrocarboxylation, and hydrogenation reactions will be discussed, finally combining the individual reaction approaches towards potential new pathways to the envisaged alcohol products. Also, tailored reactor concepts with adapted recycling/separation methods for the molecular catalyst systems will be shown and discussed.

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Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Schmitz, M. / Erken, C. / Ohligschläger, A. / Schnoor, J.‐K. / Westhues, N. F. / Klankermayer, J. / Leitner, W. / Liauw, M. A.

A detailed overview for homogeneously catalyzed strategies and synthesis pathways using a combination of CO₂, CO, and H₂ as active building blocks to selectively obtain C1–C4 alcohols is presented. Conceptual strategies applying homologation, carbonylation, hydrocarboxylation, and hydrogenation reactions will be discussed, finally combining the individual reaction approaches towards potential new pathways to the envisaged alcohol products. Also, tailored reactor concepts with adapted recycling/separation methods for the molecular catalyst systems will be shown and discussed.

Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Schmitz, M. / Erken, C. / Ohligschläger, A. / Schnoor, J.‐K. / Westhues, N. F. / Klankermayer, J. / Leitner, W. / Liauw, M. A.

A detailed overview for homogeneously catalyzed strategies and synthesis pathways using a combination of CO₂, CO, and H₂ as active building blocks to selectively obtain C1–C4 alcohols is presented. Conceptual strategies applying homologation, carbonylation, hydrocarboxylation, and hydrogenation reactions will be discussed, finally combining the individual reaction approaches towards potential new pathways to the envisaged alcohol products. Also, tailored reactor concepts with adapted recycling/separation methods for the molecular catalyst systems will be shown and discussed.

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Title:

Homogeneously Catalyzed Synthesis of (Higher) Alcohols (C1–C4) from the Combination of CO₂/CO/H₂

Contributors:

Schmitz, M. (author) / Erken, C. (author) / Ohligschläger, A. (author) / Schnoor, J.‐K. (author) / Westhues, N. F. (author) / Klankermayer, J. (author) / Leitner, W. (author) / Liauw, M. A. (author)

Published in:

Chemie Ingenieur Technik ; 90 ; 1476-1488

Publication date:

2018-10-01

Size:

13 pages

ISSN:

0009-286X , 1522-2640

DOI:

https://doi.org/10.1002/cite.201800053

Type of media:

Article (Journal)

Type of material:

Electronic Resource

Language:

English

Keywords:

Carbon2Chem® , Homogeneous catalysis , (Reverse) Water‐gas shift reaction , Alcohols , Carbon dioxide

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